A Flexible Ceramic/Polymer Hybrid Solid Electrolyte for Solid‐State Lithium...

Paper

Abstract

Abstract Ceramic/polymer hybrid solid electrolytes (HSEs) have attracted worldwide attentions because they can overcome defects by combining the advantages of ceramic electrolytes (CEs) and solid polymer electrolytes (SPEs). However, the interface compatibility of CEs and SPEs in HSE limits their full function to a great extent. Herein, a flexible ceramic/polymer HSE is prepared via in situ coupling reaction. Ceramic and polymer are closely combined by strong chemical bonds, thus the problem of interface compatibility is resolved and the ions can transport rapidly by an expressway. The as‐prepared membrane demonstrates an ionic conductivity of 9.83 × 10 −4 S cm −1 at room temperature and a high Li + transference numbers of 0.68. This in situ coupling reaction method provides an effective way to resolve the problem of interface compatibility.

Analysis

Paper intelligence

Summary

This paper presents a novel flexible ceramic/polymer hybrid solid electrolyte (HSE) prepared via an in situ coupling reaction to address interface compatibility issues in solid-state batteries.

Key findings

Resolved interface compatibility issues between ceramic and polymer components.
Achieved rapid ion transport through strong chemical bonds.
Demonstrated an ionic conductivity of 9.83 × 10⁻⁴ S cm⁻¹ at room temperature.
Obtained a high Li⁺ transference number of 0.68.

Methods

In situ coupling reaction to prepare the ceramic/polymer hybrid solid electrolyte.
Characterization of ionic conductivity and Li⁺ transference numbers.

Limitations

The abstract does not explicitly detail limitations of the study.

Applications

Solid-state lithium metal batteries.

Confidence100%

Discovery

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Source record

Publication metadata

Authors: Kecheng Pan; Lan Zhang; Weiwei Qian; Xiangkun Wu; Kun Dong; Haitao Zhang; Zhibo Zhang
Published: Mar 16, 2020
Journal or venue: Advanced Materials
DOI: 10.1002/adma.202000399
Paper type: journal article
Source: Openalex

DOI OpenAlex